In 1955 she produced the film Anarkali, in which she herself played the titular role, with Akkineni Nageswara Rao as Prince Salim. She acted in various roles, such as a damsel, an angel, a dancer, a demon, a goddess, a traditional woman and later in mother roles. In Balaiah's Police Alludu and Anna Vadina she appeared alongside Brahmanandam. Brundavanam (1992), Anna Vadina (1993) and Police Alludu (1994) were the last few films of her career. She is well known for playing Sita in Lava Kusa and her performances in films like Suvarna Sundari and Anarkali were also appreciated. She acted in Lava Kusa, a milestone film and the first color film in the Telugu film industry in 1963. She eventually acted in more than 350 films, majority of them in Telugu films and a few in Hindi, Tamil and Kannada films as the heroine or in character roles. Based on her acting ability and looks, she became a star overnight in 1947. Later, C.Pullayya discovered her and gave her the opportunity to star as Mohini in Gollabhama (1947). Prasad in 1940, but that film was abandoned after three reels shooting. Her first film as a heroine was Kashtajeevi by L. She was a theatre artiste before venturing into movies, her debut film role was as Lohitasva in ' Raja Harishchandra' in 1936. Pullaiah changed her name to Anjali Devi. She changed her name to Anjani Kumari when acting in dramas. Anjali Devi was born in Peddapuram, East Godavari district in Andhra Pradesh, India, as Anjamma.

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